B. G. Danly, R. J. Temkin
The dispersion equations are derived for two laser fields of arbitrary intensity interacting with a homogeneously broadened, three-level molecular system. The results obtained apply to laser-pumped molecular lasers and may be used to analyze frequency pulling of the emitting laser and self-focusing or defocusing of the pump laser. The present theory evaluates the dispersion function for the emitting laser in various limits, particularly focusing on cases relevant to a laser-pumped molecular laser. Notably, the analysis is also applied to previous experimental data concerning cavity frequency pulling in CO2 laser-pumped molecular lasers, including both a 385-μm D2O laser and a 496-μm CH3F laser. Good agreement is found between theory and experimental results, indicating the effectiveness of the approach in modeling the behaviors involved. In conclusion, the derived equations provide significant insights into the interaction dynamics within the laser-pumped molecular systems, highlighting the influence of intensity and resonance on dispersion phenomena.
@article{52dd550e-037e-4921-8a81-10515e29b66a,
title={Dispersion in a laser pumped molecular l},
author={B. G. Danly and R. J. Temkin},
year={2026},
language={en}
}TY - JOUR TI - Dispersion in a laser pumped molecular l AU - B. G. Danly AU - R. J. Temkin PY - 2026 LA - en ER -
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