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2026 Liu Calcium impurity control in manganese sulfate solution

Jiajie Liu, Zong Guo

2026ensolvent extractioncalcium removalmanganese sulfatebattery recyclingorganophosphorus extractantlithium batteries

Abstract

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To address the difficulty of efficiently removing calcium impurities from the manganese sulfate stripping solution obtained during the recycling of spent lithium batteries, this work proposed a binary synergistic extraction system. Quantum chemical calculations were used to screen the optimal combination (2A + 2B). The binding energy indicated the molecules combined with calcium are relatively more stable. Experimental optimization determined the optimal conditions as follows: 50 vol% of A, 25 vol% of B, saponification rate 60%, phase ratio (O/A) 2.5:1, and pH 6.0. In continuous extraction tank experiments, the calcium concentration decreased from 681 mg/L to 5 mg/L after a seven-stage counter-current extraction, with an extraction efficiency of about 99.3%. Infrared spectroscopy confirmed that the P=O double bond was the key functional group. This study provides an efficient and feasible technological pathway for the preparation of battery-grade manganese sulfate.

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Cite This Work

@article{a296c358-fbd2-444b-837a-d40bc30fd302,
  title={2026   Liu   Calcium impurity control in manganese sulfate solution},
  author={Jiajie Liu and Zong Guo},
  year={2026},
  language={en}
}
TY  - JOUR
TI  - 2026   Liu   Calcium impurity control in manganese sulfate solution
AU  - Jiajie Liu
AU  - Zong Guo
PY  - 2026
LA  - en
ER  -

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